Roldós is a surname. Notable people with the surname include:
Jaime Roldós Aguilera (1940–1981), President of Ecuador (1979–81) León Roldós Aguilera (born 1942), Vice President of Ecuador (1981–1984) Martha Roldós (born 1963), Ecuadorian economist and politician, daughter of Jaime Mercedes Roldós Freixes (1910–1989), Spanish composer and music educator