Wolle is a German surname meaning "wool". Notable people with the surname include:

Arno Wolle (1903–1988), Danish naturopath and mathematician Charles R. Wolle (1935–2022), American jurist from Iowa; former federal judge of the U. S. district court Christian Jacob Wolle (1788–1863), American plant collector and innkeeper Francis Wolle (1817–1893), American priest of the Moravian Church Gertrud Wolle (1891–1952), German film actress Muriel Sibell Wolle (1898–1977), American artist; known for paintings of mining communities Robert H. Wolle, Sr. (1924–2017), American environmentalist and public health pioneer Stefan Wolle (born 1950), German historian William D. Wolle (born 1928), American foreign service officer and ambassador