Walrond is a surname. Notable people with the surname include:
Edmund Walrond (1655–1708), English Member of Parliament Emma Maria Walrond (1859–1943), New Zealand painter Eric D. Walrond (1898–1966), Harlem Renaissance writer Humphrey Walrond (c. 1600 – c. 1670), deputy governor of Barbados Sir John Walrond (1818-1889), British politician Les Walrond (b. 1976), American baseball player Violet Walrond (1905–1996), New Zealand Olympic swimmer William Walrond, 1st Baron Waleran (1849–1925), British peer William Walrond (politician) (1876–1915), Member of Parliament; son of the above