Toland is a surname. Notable people with the surname include:
Brook Toland (born 1992), American actress Christopher Toland (born 1985), American figure skater George Washington Toland (1796–1869), American politician Gregg Toland (1904–1948), American cinematographer Hugh Toland (1806–1880), American surgeon and academic John Toland (1670–1722), Irish-born rationalist philosopher and freethinker John Toland (born 1949), Irish mathematician John Toland (1912–2004), American author and historian Lee Toland Krieger (born 1983), American film director M. B. M. Toland (1925-1895), American poet and social leader; wife of Hugh Toland Mark Toland (born 1986), American magician Tank Toland (born 1973), American wrestler Tyler Toland (born 2001), Irish football player